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Research Article

Evidence of neutron leakage at the Fukushima nuclear plant from measurements of radioactive 35S in California

Antra Priyadarshi, Gerardo Dominguez, and Mark H. Thiemens
  1. 9500 Gilman Drive, University of California, San Diego, La Jolla, CA 92093

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PNAS August 30, 2011 108 (35) 14422-14425; https://doi.org/10.1073/pnas.1109449108
Antra Priyadarshi
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Gerardo Dominguez
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Mark H. Thiemens
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  • For correspondence: mthiemens@ucsd.edu
  1. Edited* by Karl K. Turekian, Yale University, North Haven, CT, and approved July 18, 2011 (received for review June 10, 2011)

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    Fig. 1.

    35S activity measured in SO2 gas and sulfate aerosol collected at SIO, La Jolla. A significant increase in Embedded Image concentration was observed on March 28, 2011, from the natural background Embedded Image activity. The higher activity observed at SIO is due to the presence of higher concentration of Embedded Image (365 times higher than the natural abundance) at Fukushima and the radiation plume being transported over the Pacific.

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    Fig. 2.

    Ten-day back trajectory obtained for the air mass reaching La Jolla, California, on March 28, 2011, from HYSPLIT model indicates that the air mass originated at Japan.

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    Fig. 3.

    Schematic description of a moving box model developed to calculate the concentration of Embedded Image and Embedded Image at Scripps pier, La Jolla (California) due to the long-range transport of radiation plume from Fukushima. The atmosphere is divided into four layers: MBL, BuL, free troposphere (FT), and lower stratosphere (LS). τdill is the dilution lifetime of the radiation plume. τox is the oxidation lifetime of Embedded Image, whereas τc and τd are the cloud scavenging and dry depositional lifetime of Embedded Image, respectively. τr is the removal lifetime of Embedded Image (see SI Text). The dotted line (red) represents the mean transit altitude at which air mass transport occurred; it was calculated from HYSPLIT model. The model parameters in the box were changed according to its transit altitude (Table S3).

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    Table 1.

    The measurements of 35S activity contained in SO2 (gas) and sulfate aerosol collected at Scripps, La Jolla, California, during March–April 2011

    SampleTotal air flow, m3 Total disintegration per minute (measured)35S, atoms/m3Total [Embedded Image], ng/m3
    Start dateEnd date
    Embedded Image
    3-2-20113-9-201113,26918.0 ± 0.4246 ± 23.8
    3-9-20113-15-20119,51812.9 ± 0.3246 ± 36.6
    3-15-20113-17-20113,3383.3 ± 0.2180 ± 66.1
    3-17-20113-22-20117,81910.4 ± 0.3241 ± 318.8
    3-22-20113-24-20113,47916.8 ± 0.3876 ± 74.8
    3-24-20113-28-20116,50253.8 ± 0.41501 ± 53.9
    3-28-20114-1-20116,3947.4 ± 0.2210 ± 36.5
    4-1-20114-5-20116,51111.5 ± 0.3320 ± 410.6
    4-5-20114-8-20114,80212.6 ± 0.3475 ± 59.3
    4-8-20114-12-20116,4378.4 ± 0.3237 ± 45.5
    Embedded Image
    3-15-20113-17-20113,3381.2 ± 0.130 ± 61.3
    3-17-20113-22-20117,8193.3 ± 0.180 ± 31.4
    3-22-20113-24-20113,4791.7 ± 0.1100 ± 60.9
    3-24-20113-28-20116,5024.3 ± 0.1120 ± 30.8
    3-28-20114-1-20116,3941.8 ± 0.150 ± 31.9
    4-1-20114-5-20116,5111.0 ± 0.128 ± 21.0
    4-5-20114-8-20114,8021.4 ± 0.152 ± 31.0
    4-8-20114-12-20116,4371.4 ± 0.141 ± 31.2

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Evidence of neutron leakage at the Fukushima nuclear plant from measurements of radioactive 35S in California
Antra Priyadarshi, Gerardo Dominguez, Mark H. Thiemens
Proceedings of the National Academy of Sciences Aug 2011, 108 (35) 14422-14425; DOI: 10.1073/pnas.1109449108

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Evidence of neutron leakage at the Fukushima nuclear plant from measurements of radioactive 35S in California
Antra Priyadarshi, Gerardo Dominguez, Mark H. Thiemens
Proceedings of the National Academy of Sciences Aug 2011, 108 (35) 14422-14425; DOI: 10.1073/pnas.1109449108
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Proceedings of the National Academy of Sciences: 108 (35)
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