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Research Article

Charge separation and charge delocalization identified in long-living states of photoexcited DNA

Dominik B. Bucher, Bert M. Pilles, Thomas Carell, and Wolfgang Zinth
  1. aBioMolecular Optics and Center for Integrated Protein Science, Ludwig-Maximilians-Universität München, 80538 Munich, Germany; and
  2. bCenter for Integrated Protein Science, Department of Chemistry, Ludwig-Maximilians-Universität München, 81377 Munich, Germany

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PNAS March 25, 2014 111 (12) 4369-4374; https://doi.org/10.1073/pnas.1323700111
Dominik B. Bucher
aBioMolecular Optics and Center for Integrated Protein Science, Ludwig-Maximilians-Universität München, 80538 Munich, Germany; and
bCenter for Integrated Protein Science, Department of Chemistry, Ludwig-Maximilians-Universität München, 81377 Munich, Germany
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Bert M. Pilles
aBioMolecular Optics and Center for Integrated Protein Science, Ludwig-Maximilians-Universität München, 80538 Munich, Germany; and
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Thomas Carell
bCenter for Integrated Protein Science, Department of Chemistry, Ludwig-Maximilians-Universität München, 81377 Munich, Germany
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  • For correspondence: wolfgang.zinth@physik.uni-muenchen.de thomas.carell@cup.uni-muenchen.de
Wolfgang Zinth
aBioMolecular Optics and Center for Integrated Protein Science, Ludwig-Maximilians-Universität München, 80538 Munich, Germany; and
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  • For correspondence: wolfgang.zinth@physik.uni-muenchen.de thomas.carell@cup.uni-muenchen.de
  1. Edited by Mark Ratner, Northwestern University, Evanston, IL, and approved February 19, 2014 (received for review December 20, 2013)

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Article Information

vol. 111 no. 12 4369-4374
DOI: 
https://doi.org/10.1073/pnas.1323700111
PubMed: 
24616517

Published By: 
National Academy of Sciences
Print ISSN: 
0027-8424
Online ISSN: 
1091-6490
History: 
  • Published in issue March 25, 2014.
  • Published first March 10, 2014.


Author Information

  1. Dominik B. Buchera,b,
  2. Bert M. Pillesa,
  3. Thomas Carellb,1, and
  4. Wolfgang Zintha,1
  1. aBioMolecular Optics and Center for Integrated Protein Science, Ludwig-Maximilians-Universität München, 80538 Munich, Germany; and
  2. bCenter for Integrated Protein Science, Department of Chemistry, Ludwig-Maximilians-Universität München, 81377 Munich, Germany
  1. Edited by Mark Ratner, Northwestern University, Evanston, IL, and approved February 19, 2014 (received for review December 20, 2013)

Footnotes

  • ↵1To whom correspondence may be addressed. E-mail: wolfgang.zinth{at}physik.uni-muenchen.de or thomas.carell{at}cup.uni-muenchen.de.
  • Author contributions: D.B.B. and W.Z. designed research; D.B.B. and B.M.P. performed research; D.B.B., T.C., and W.Z. analyzed data; and D.B.B., T.C., and W.Z. wrote the paper.

  • The authors declare no conflict of interest.

  • This article is a PNAS Direct Submission.

  • This article contains supporting information online at www.pnas.org/lookup/suppl/doi:10.1073/pnas.1323700111/-/DCSupplemental.

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Photoexcitation of DNA leads to charge separation
Dominik B. Bucher, Bert M. Pilles, Thomas Carell, Wolfgang Zinth
Proceedings of the National Academy of Sciences Mar 2014, 111 (12) 4369-4374; DOI: 10.1073/pnas.1323700111

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Photoexcitation of DNA leads to charge separation
Dominik B. Bucher, Bert M. Pilles, Thomas Carell, Wolfgang Zinth
Proceedings of the National Academy of Sciences Mar 2014, 111 (12) 4369-4374; DOI: 10.1073/pnas.1323700111
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Proceedings of the National Academy of Sciences: 111 (12)
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