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Local quantum phase transition in YFe2Al10

W. J. Gannon, L. S. Wu, I. A. Zaliznyak, W. H. Xu, A. M. Tsvelik, Y. Qiu, J. A. Rodriguez-Rivera, and M. C. Aronson
PNAS July 3, 2018 115 (27) 6995-6999; published ahead of print June 18, 2018 https://doi.org/10.1073/pnas.1721493115
W. J. Gannon
aDepartment of Physics and Astronomy, Texas A&M University, College Station, TX 77843-4242;
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  • For correspondence: wgannon@physics.tamu.edu
L. S. Wu
bNeutron Scattering Division, Oak Ridge National Laboratory, Oak Ridge, TN 37831;
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I. A. Zaliznyak
cCondensed Matter Physics and Materials Science Division, Brookhaven National Laboratory, Upton, NY 11973;
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  • ORCID record for I. A. Zaliznyak
W. H. Xu
cCondensed Matter Physics and Materials Science Division, Brookhaven National Laboratory, Upton, NY 11973;
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A. M. Tsvelik
cCondensed Matter Physics and Materials Science Division, Brookhaven National Laboratory, Upton, NY 11973;
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Y. Qiu
dNational Institute of Standards and Technology Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, MD 20899;
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J. A. Rodriguez-Rivera
dNational Institute of Standards and Technology Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, MD 20899;eDepartment of Materials Science and Engineering, University of Maryland, College Park, MD 20740
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M. C. Aronson
aDepartment of Physics and Astronomy, Texas A&M University, College Station, TX 77843-4242;
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  1. Edited by Subir Sachdev, Harvard University, Cambridge, MA, and approved May 9, 2018 (received for review December 13, 2017)

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Significance

We report the discovery of a type of phase transition that occurs at T=0. In continuous phase transitions, order occurs when the size and lifetime of small ordered regions increase until they span the system and become static. Reported here is experimental evidence of a transition where this paradigm fails. Our observed phase transition is local, where each magnetic moment in YFe2Al10 is independent of every other moment, yet each moment follows the same spectrum of quantum critical fluctuations. The phase transition present in YFe2Al10 is a realization of a scenario only hinted at by theory, corresponding to the formation of magnetic moments, with no evidence for the breaking of translational symmetry that accompanies magnetic order.

Abstract

A phase transition occurs when correlated regions of a new phase grow to span the system and the fluctuations within the correlated regions become long lived. Here, we present neutron scattering measurements showing that this conventional picture must be replaced in YFe2Al10, a compound that forms naturally very close to a T=0 quantum phase transition. Fully quantum mechanical fluctuations of localized moments are found to diverge at low energies and temperatures; however, the fluctuating moments are entirely without spatial correlations. Zero temperature order in YFe2Al10 is achieved by an entirely local type of quantum phase transition that may originate with the creation of the moments themselves.

  • magnetism
  • quantum matter
  • neutron scattering

Footnotes

  • ↵1To whom correspondence should be addressed. Email: wgannon{at}physics.tamu.edu.
  • ↵2Department of Physics, South University of Science and Technology of China, Shenzhen, 518055, China.

  • Author contributions: W.J.G., L.S.W., and M.C.A. designed research; W.J.G., L.S.W., I.A.Z., W.H.X., A.M.T., Y.Q., J.A.R.-R., and M.C.A. performed research; W.J.G. analyzed data; and W.J.G., L.S.W., I.A.Z., W.H.X., A.M.T., Y.Q., J.A.R.-R., and M.C.A. wrote the paper.

  • The authors declare no conflict of interest.

  • This article is a PNAS Direct Submission.

  • This article contains supporting information online at www.pnas.org/lookup/suppl/doi:10.1073/pnas.1721493115/-/DCSupplemental.

Published under the PNAS license.

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Local quantum phase transition in YFe2Al10
W. J. Gannon, L. S. Wu, I. A. Zaliznyak, W. H. Xu, A. M. Tsvelik, Y. Qiu, J. A. Rodriguez-Rivera, M. C. Aronson
Proceedings of the National Academy of Sciences Jul 2018, 115 (27) 6995-6999; DOI: 10.1073/pnas.1721493115

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Local quantum phase transition in YFe2Al10
W. J. Gannon, L. S. Wu, I. A. Zaliznyak, W. H. Xu, A. M. Tsvelik, Y. Qiu, J. A. Rodriguez-Rivera, M. C. Aronson
Proceedings of the National Academy of Sciences Jul 2018, 115 (27) 6995-6999; DOI: 10.1073/pnas.1721493115
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