Conservation laws and the foundations of quantum mechanics

Contributed by Yakir Aharonov; received December 9, 2022; accepted July 31, 2023; reviewed by Lucien Hardy and Serge Massar
October 2, 2023
120 (41) e2220810120

Significance

Conservation laws are some of the most important laws of physics. Having their origin in the symmetries of nature, conservation laws are present in all our physical theories. There are, however, significant differences between what conservation laws mean in these various theories. In quantum mechanics, which is a theory that is nondeterministic at a fundamental level, the conservation laws, as they are standardly formulated, do not refer to individual experiments but only to the statistics over a large ensemble of repeated identical experiments. Here, we take a step toward extending quantum conservation laws to individual cases.

Abstract

In a recent paper, [Y. Aharonov, S. Popescu, D. Rohrlich, Proc. Natl. Acad. Sci. U.S.A.118 e1921529118 (2021)], it was argued that while the standard definition of conservation laws in quantum mechanics, which is of a statistical character, is perfectly valid, it misses essential features of nature and it can and must be revisited to address the issue of conservation/nonconservation in individual cases. Specifically, in the above paper, an experiment was presented in which it can be proven that in some individual cases, energy is not conserved, despite being conserved statistically. It was felt however that this is worrisome and that something must be wrong if there are individual instances in which conservation does not hold, even though this is not required by the standard conservation law. Here, we revisit that experiment and show that although its results are correct, there is a way to circumvent them and ensure individual case conservation in that situation. The solution is however quite unusual, challenging one of the basic assumptions of quantum mechanics, namely that any quantum state can be prepared, and it involves a time-holistic, double nonconservation effect. Our results bring light on the role of the preparation stage of the initial state of a particle and on the interplay of conservation laws and frames of reference. We also conjecture that when such a full analysis of any conservation experiment is performed, conservation is obeyed in every individual case.
Conservation laws are some of the most important laws of physics. Having their origin in the symmetries of nature, conservation laws are present in all our physical theories, from classical mechanics, to relativistic and quantum physics. There are, however, significant differences between what conservation laws mean in these various theories. In quantum mechanics, which is a theory that is nondeterministic at a fundamental level, conservation laws have a different manifestation than in classical mechanics. Indeed, in classical mechanics, in each run of an experiment, we can determine the initial value of the conserved quantity and at the end of the experiment, we can check that its final value is identical to it. On the other hand, in quantum mechanics where the initial state of a system may not have a well-defined value for the conserved quantity, but some superposition of it, and the outcome of the final measurement cannot, in general, be predicted from the knowledge of the initial state, one cannot directly apply the same concept of “conservation” as in classical physics. In face of these difficulties, the concept of conservation that applies to classical mechanics was generalized: The standard definition of conservation used at present in quantum mechanics is statistical.
However, in a recent paper (1) based on ideas first formulated in ref. 2, we have argued that while the statistical definition is perfectly valid as far as it goes—and it is an extremely useful concept—it misses essential features of nature and has to be revisited and extended. Ref. 1 however did not go further than pointing out the need for this revision and did not offer a “solution.” Here, we show that taking this idea seriously leads to uncovering some extremely surprising phenomena and challenges one of the basic assumptions of quantum mechanics, namely that any quantum state can be prepared.
The argument in ref. 1 stems from the discovery of a particular situation that challenges the standard view. In particular, we have described there a situation in which a box contains a single particle prepared in a state |Ψ which is a superposition of energy eigenstates, with all energies less than a maximal value Emax. In some runs of the experiment, the particle emerges from the box. When it does this, it emerges with an energy much higher than Emax, the maximal energy component present in its initial state, all this while the mechanical system used for extracting the particle—the only other system in the problem—does not change its state to account for this energy change. Hence, in the individual cases when the particle emerges from the box, energy is not to be conserved. Similar examples can also be constructed for other conserved quantities such as momentum and angular momentum. So what does this example tell us?
The above example, surprising as it is, is not in contradiction with the standard definition of conservation laws in quantum mechanics. Quantum conservation laws are statistical, and they refer to many (theoretically infinite) repeated experiments and to the probabilities of the outcomes of these measurements. More precisely, according to the standard definition of conservation laws in quantum mechanics, a quantity is said to be conserved if the following is the case: If we prepare an ensemble of systems in the same initial state and immediately after the preparation we measure the quantity of interest, we obtain the same probability distribution of the outcomes as when we first let the systems evolve and we measure this quantity only after the end of the experiment. What is essential in this definition is that it refers to the entire ensemble. In our example, if we were to count all runs of the experiment, both those in which the particle emerges out of the box and those in which it did not, we find that the standard conservation law holds. (After all, it is impossible to be otherwise, by the very way in which conservation laws are defined: When a quantity commutes with the Hamiltonian—the only situation when the dynamics is such that quantity should be conserved—the standard conservation law always holds true.)
The problem is that the standard conservation law tells nothing about individual cases. Imagine however that the box contained a particle of energy of order 1 eV (more precisely a particle in a superposition of various energies but absolutely none of them larger than 1 eV) and that in one run of the experiment when we open the box the particle emerges with energy of order of millions of GeV, while the mechanism that extracted the particle from the box, the only other system in the problem, did not change its state. It seems legitimate to worry about what’s going on. To us, it seems that something must be wrong if there are individual instances in which conservation does not hold, even if over the entire statistical ensemble of cases conservation holds.
Here, we revisit the experiment of ref. 1 and present the solution to that problem. The solution involves two elements: First, we avoid the individual-case nonconservation problem presented in ref. 1 by arguing that its setting is unphysical, challenging therefore one of the basic assumptions of quantum mechanics, namely that any quantum state can be prepared. Second, we show that modifying the experiment to make it physical implies that actually there is conservation in the individual case we consider. This happens via a time-holistic, double nonconservation effect. Our results bring light on the role of the preparation stage of the initial state of a particle, as well as on the interplay of conservation laws and frames of reference. We also conjecture that when such a full analysis of any conservation experiment is performed conservation is obeyed in any individual case, not only statistically.
The paper is organized as follows. We start (the first four sections) by recalling the arguments of ref. 1 for the need to revisit the issue of conservation laws. We then set the stage (by presenting the basic effect discussed in ref. 1 but reformulated for the case of angular momentum conservation, which is much simpler as it avoids the complications of time evolution. While the case of angular momentum conservation has been discussed briefly also in an appendix (1), here, we give more details which are essential for understanding the results. The next three sections introduce our basic conceptual element and present the main result of the paper. The rest of the paper is devoted to Discussions and Conclusions.

Superoscillations

It is useful to start by recalling the basic experiment in more detail.
At the core of our examples is the function f(x)
f(x)=1+α2eix/N+1α2eix/NN,
[1]
with N an integer that we will take as large as we want and with α a real constant with the crucial property that α>1.
This function has the property of “superoscillations”; see refs. 1 and 2) as well as (35) and the extensive review (6). It is a widespread belief that a function cannot have features smaller than the smallest wavelength of its Fourier components. Yet this is not true, as shown in refs. 1 and 2. Superoscillatory functions can oscillate on arbitrary long intervals with much shorter wavelengths than any of their Fourier components. Or, in frequency terms, they can oscillate with much higher frequency than the highest Fourier component. In particular, the function f(x) in Eq. 1 is a superposition of frequencies strictly limited to the interval [1,1]. However, for large N, in the region |x| of order of N12ϵ where ϵ is an arbitrary small fixed positive constant, the function is
f(x)eiαx,
[2]
that is, it oscillates with frequency α>1, faster than the maximal Fourier component.
To prove the above claims, first, by expanding the binomial, we see that f(x) is a superposition of Fourier components of frequencies 2nNN, with n integer, 0nN, which are limited to the interval [1,1]:
f(x)=n=0NCnei2nNNx,
[3]
with Cn constants
Cn=Nn(1+α2)n(1α2)Nn.
[4]
However, consider now this function in the region |x|L where L is some fixed number, and let N increase. (This is a smaller region than N12ϵ where the superoscillations hold, but here, the proof is immediate. For the larger region of order N12ϵ, see ref. 1 as well as SI Appendix, Supporting Information I.) For large N, up to corrections of order O(1/N), we can approximate the exponentials by their first-order Taylor expansion and obtain
f(x)1+α2(1+ixN)+1α2(1ixN)N=1+iαxNNeiαx,
[5]
which means that in this region, the function oscillates with frequency α.
Finally, note that since the size of the superoscillatory region increases with N, the number of superoscillatory wavelengths λ=2πα in the superoscillatory region can be made as large as we want by taking N large enough.

The Experiment

In the present paper, we will focus on angular momentum conservation, since it is somewhat simpler than the energy nonconservation example of ref. 1, though it is constructed along very similar lines.
For simplicity, we will also consider the mass of the particle of interest to be large enough and the time scales short enough so that the free Hamiltonian of the particle can be neglected.
We now construct our basic experiment using a version of the superoscillatory function f. Consider a particle moving on a circle and let θ, πθπ, denote its position. Let the wavefunction be |Ψ which in the angle representation is
Ψ(θ)=N1+a2eiθ+1a2eiθN,
[6]
where a is an integer larger than 1 and N is a normalization factor. (The restriction of a to integers is made for mathematical simplicity; the conclusions will not change if we take a to be any rational or real number larger than 1).
Consider now the region of small angles |θ| of order 1/N1/2+ϵ. As we increase N, in this region, the state Ψ(θ) presents superoscillations. The proof is immediate:
Since we will only be interested in angular momentum, once the angular dependence of the wavefunction is given, the value of the radius of the circle is irrelevant. However, it is convenient (also with an eye to possible experiments) to think of a circle of radius RN=Nr0 with r0 a fixed length. The region of interest, |θ|=O(1/N1/2+ϵ), corresponds to an arc length L along the circle of order N1/2ϵr0. In the variable x=θRN that denotes the position along the circle, the situation maps immediately to that investigated in Eqs. 12; we can re-express it afterward in term of angles.
Following the same calculation as in Eq. 12, we find that Ψ(θ) is a superposition of angular momentum eigenstates eimθ of the angular momentum operator L̂ of eigenvalues m, with NmN (where we take ħ=1):
Ψ(θ)=Nn=0NCnei(2nN)θ=Nm=NNcmeimθ,
[7]
where Cn is given by Eq. 4 with α=a and where cm=C2nN.
On the other hand, for |θ| of order 1/N1/2+ϵ, in the limit of large N,
Ψ(θ)NeiaNθ,
[8]
a much higher angular frequency, mimicking in this region a particle with angular momentum aN, a times higher than the highest angular momentum in the superposition. Note also that if we take N large enough, we can have the superoscillatory region to extend for as many superoscillatory wavelengths as we want.
The experiment consists in determining if the particle is in the superoscillatory region. In technical terms, we want to measure the projector on that region. When we find the particle there, it has angular momentum of approximately aN, which is much higher than all the angular momentum components that it initially had. The question is where did it take supplementary angular momentum from?

The Paradox

It is tempting to think that the answer is trivial and straightforward: There are two systems in the problem—the particle and the measuring device used for measuring the position. They interact when the measurement takes place. As the particle increased its angular momentum, surely, it must have received a kick from the measuring device. In return, the measuring device must have decreased its own angular momentum. Hence, this seems nothing else than a trivial example of conservation of the total angular momentum. Only that it is not so: The measuring device could not have provided the necessary angular momentum. In fact, in the limit of large N, the measuring device did not change its state at all.
The argument is simple. Let us compare what happens in two cases: i) when measurements are made on the particle prepared in the superoscillatory state |Ψ which mimics the high angular momentum aN in the region of interest and ii) when measurements are performed on a particle prepared in an angular momentum eigenstate of eigenvalue aN, i.e., when the high angular momentum is genuine. The interaction between the measuring device and the particle takes place in the region of superoscillations. In this region, the particle’s wavefunction |Ψ looks (up to perturbations that we can make as small as we want by choosing N large enough) like the eigenstate of angular momentum with value aN. Suppose now that we perform a measurement of the projection operator on the superoscillatory region. Since the difference between the wavefunction Ψ and the true eigenstate of eigenvalue aN is only encoded in the wavefunction outside the superoscillatory region and since we took the free Hamiltonian of the particle to be zero which means that this information cannot propagate, this information is unavailable to the measuring device and cannot affect the result. Hence, the measuring device will behave in the same way in both cases.
Let us compare these two cases. In the latter case, the wavefunction is a monochromatic wave of wavelength λ=2πRN/aN=2πr0/a (corresponding to the angular momentum aN). All that happens when we find the particle in our region of interest, |x| of order N1/2ϵr0, is that the measuring devices simply cuts out of this monochromatic wave a wave-train of length equal to the lengths of this region. Since for increasing N, this region contains more and more wavelengths, this wave-train approximates better and better the original monochromatic wave. In other words, if we find the particle in the region of interest, the final wavefunction has angular momentum closer and closer to the original high angular momentum, and hence, the measuring device does not give it any supplementary angular momentum at all. But then, the measuring device could not give angular momentum in the first case either, since in both cases, it must behave in the same way. This is the paradox.

Modeling the Measurement

To model the measurement of the projection operator onto the region of interest in such a way as to enable us to see the exchange of angular momentum between the system and the measuring device, we proceed as follows. We take the measuring device to be a second particle which also moves on the circle and which has an internal degree of freedom of this particle, the “pointer.” The location of the measuring device on the circle determines the location of the region where we would like to perform the projection. Let its coordinate be denoted by θM, and let its initial wavefunction be ϕ(θM). Let the pointer consist of an internal degree of freedom described by a 2-dimensional Hilbert space. Initially, we take the pointer in the state |. The initial state of the particle and measuring device is therefore
Ψ(θ)ϕ(θM)|.
[9]
What we want to arrange is an interaction that a) conserves the total angular momentum and b) the pointer flips to state | if and only if the particle is in the superoscillatory region. We can do this by using the interaction Hamiltonian
H=π2δ(t)g(θθM;φ)σx,
[10]
where g(θ;φ) denotes a square pulse of width φ, with 0<φ<π/2, i.e.,
g(θ;φ)=1forθmod2πφ0forθmod2πφ,
[11]
and where the σx operator flips to and vice-versa.
Note first that the angular dependence of the Hamiltonian is only via (θθM)mod2π, the relative angle between the particle and the measuring device. This ensures conservation of the total angular momentum. Second, the Hamiltonian is zero for (θθM)mod2πφ and proportional to σx for (θθM)mod2πφ. In other words, it flips the pointer only when the particle is within a distance φ from θM, the location of the measuring device, and leaves the pointer unchanged when the particle is further away. All that is left is to take φ and θM such as to ensure that this region is within the superoscillatory region and captures as much as possible of this region. To do this, we take φ of the order of the superoscillatory region and prepare the measuring device in a wavepacket ϕ(θM) centered on θM=0 and with an appropriately small spread Δ. For example, we take (up to normalization) ϕ(θM)=g(θM;Δ) with Δ<<φ, so that the interval |θ||φ+Δ| is still in the superoscillatory region.
The corresponding unitary time evolution operator over an infinitesimal time τ is
Û(τ,0)=ei0τĤ(t)dt=eiπ2g(θθM;φ)σx=cos(π2g(θθM;φ))+iσxsin(π2g(θθM;φ))=1g(θθM;φ)+ig(θθM;φ)σx,
[12]
where in the last equality, we used in the trigonometric functions the definition of the function g.
For any arbitrary initial state ψ(θ) of the particle, the state of the particle and the measuring device is a superposition of two terms, one with the pointer flipped (for (θθM)mod2πφ) and one with the pointer not flipped:
ψ(θ)ϕ(θM)|Ûψ(θ)ϕ(θM)|=(1g(θθM;φ))ψ(θ)ϕ(θM)|+ig(θθM;φ)ψ(θ)ϕ(θM)|.
[13]
As expected, the term with the flipped pointer is (up to normalization) simply the arbitrary original state ψ truncated to a region of size φ centered on θM, that is, the projection of the original state onto this region.
Let’s now take the arbitrary state ψ to be the superoscillatory state Ψ. In this case, when the pointer has flipped, the state of the particle and measuring device is (up to normalization)
ig(θθM;φ)Ψ(θ)ϕ(θM)=ig(θθM;φ)(eiaNθ+O(1N))ϕ(θM),
[14]
using the approximation of Ψ for the small angles and the fact that for larger angles g(θθM;φ)=0.
The crucial thing, as we explained above in the previous section, is that when the particle was found in the superoscillatory region, particle plus measuring device state is, up to approximations of 1/N which can be made as small as we want, the same as when the initial state of the particle was the genuine high angular momentum eigenstate eiaNθ. So whatever happens to the measuring device when the initial state is the bona fide high angular momentum state, happens also when the initial state is our “fake” high angular momentum state.
Let us now study the particle-measuring device angular momentum exchange. Consider first what would happen if the particle were to start in the high angular momentum state aN and the measuring device pointer is flipped, meaning that the particle is found in the |θ| region where our function Ψ superoscillates. To see the angular momentum exchange in this situation, we decompose the interaction term g(θθM;φ) in its Fourier transform and obtain
g(θθM;φ)eiaNθϕ(θM)=k=sinc(kφ)eik(θθM)eiaNθϕ(θM)=k=sinc(kφ)ei(aN+k)θeikθMϕ(θM),
[15]
where we used
g(θ;φ)=k=sinc(kφ)eikθ.
[16]
Here ei(aN+k)θ is an eigenstate of the angular momentum of the particle corresponding to the eigenvalue aN+k and eikθMϕ(θM) if a state that is identical to |ΦM, the initial state of the measuring device, but shifted down in angular momentum by k.
In the Dirac notation that will be more convenient in the next sections, for the cases when the particle is found in the superoscillatory region (i.e., the measuring device pointer is flipped), the measurement time evolution is given by
|aNp|ΦMk=sinc(kφ)|aN+kp|ΦkM,
[17]
where by |ΦkM, we denote a state that is identical to |ΦM, the initial state of the measuring device, but shifted down in angular momentum by k.
What Eqs. 15 and 17 show is that in the case when initially the particle was prepared in the high angular momentum aN and it emerges from the measurement with exactly the same angular momentum aN, (that is, corresponding to k=0 Eq. 17) the measuring device does not change its angular momentum at all. This is very much expected: Since the particle did not change its angular momentum, there is no reason for the measuring device to provide it any supplementary angular momentum, so no change of the angular momentum of the measuring device should occur. When the particle emerges with other angular momentum value aN+k with k0, which occurs due to the truncation of the initial monochromatic wavefunction, the measuring device changes its angular momentum by k to compensate for the change. In other words, nothing changes in the measuring device when the particle emerges with precisely the high angular momentum aN; there are only changes to account for the deviations of the particle’s angular momentum from this value. Incidentally, we also note that these truncation disturbances become relatively less and less important with increasing N, since while the central angular momentum value increase as aN, the only significant deviations from it are only of order |k|=O(N1/2ϵ).
Now, had the particle started in our initial state Ψ, the measuring device would have reacted in the same way, up to corrections of 1/N as described in Eq. 14, so when found in the superoscillatory region, we have
|Ψp|ΦMk=sinc(kφ)|aN+kp|ΦkM+O(1N).
[18]
This means, in particular, that up to 1/N corrections, when the particle emerges with the high angular momentum value aN (with a>1), the measuring device does not provide any angular momentum to the particle, despite the fact that maximal initial angular momentum of the particle is only N. Where does the difference aNN come from in this case? This is our paradox.
The following sections give the solution.

Preparation

Let us now discuss a seemingly unrelated issue: How is this special state of the particle prepared in the first place? The reason the preparation is not completely trivial is that we are dealing with a conserved quantity, and that imposes some constraints.
In our original paper (1), we started by discussing a box containing a photon prepared in a similar special superposition of energy eigenstates. Presumably, a laser should have been employed to deliver the photon into the box. But the total energy is a conserved quantity; hence, when the laser emits the photon with a certain energy, the laser must lose the same amount. (Note: Actually, in general, the laser is connected to other objects—optical table, external power supply. It is the energy of this whole system that changes to compensate the change in the energy of the photon. For simplicity, here, we call “laser” this entire system).
As the photon is in a superposition of energy eigenstates, the laser will get entangled with it, each energy eigenstate of the photon being correlated to another state of the laser, shifted down in energy by the energy lost to the photon. The state of the photon is thus not a pure state, as we desired. However, if the state of the laser has a wide and smooth enough distribution of energy, a shift in energy does not modify the state considerably, and the entanglement is minimal. This is how nonmonochromatic but almost pure states of light are routinely prepared. In our present case, we could similarly imagine a “preparing device,” moving on the same circle as the particle, and isolated from everything else, that releases the particle on the circle that we consider. Or, for greater simplicity, imagine that we start with the particle in the initial state of zero angular momentum |0p and the preparer boosts its angular momentum appropriately. Angular momentum being a conserved quantity, the state of the preparer also changes. Again, the particle and the preparing device get entangled. Nevertheless, by choosing the initial state of the preparation device appropriately, we can make this entanglement arbitrarily small.
In other words, instead of preparing the pure state
|Ψp=m=NNcm|mp,
[19]
what the actual preparation procedure does is to take the initial particle-preparer state |0p|ΦP to the final, entangled state |χp,P, via the angular momentum conserving transformation
|0p|ΦP|χp,P=m=NNcm|mp|ΦmP,
[20]
where |ΦmP is the initial state of the preparer shifted down in angular momentum by m.
As discussed above, to make the reduced density matrix of the photon in the two-party entangled state [20] approximate that corresponding to the pure state Ψ, we need to choose the initial state of the preparer, |ΦP, as a wide and smooth enough superposition of angular momentum so that for all m, with NmN the shifted states |ΦmP are almost identical to the initial state |ΦP (i.e., PΦm|ΦP1). To achieve this goal, we take |ΦP to be narrow in its angular distribution. Indeed, the angle θP that denotes the location of the preparer is conjugated to its angular momentum, so a narrow distribution of θP ensures a wide and smooth distribution of angular momentum.
Going beyond the above purely mathematical argument of why we want to take ΦP(θP) with a narrow distribution of θP, here are two physical reasons.
First, since total angular momentum is conserved, the Hamiltonian cannot depend on the absolute value of the angle of the particle or of the preparing device but only on their relative angle θθP. Hence, to each value of θP corresponds a wavefunction of the particle appropriately shifted in space. This, of course, means entanglement between the particle and the preparing device, which we want to avoid. To limit this entanglement, we need to reduce the uncertainty in θP, hence to take for the state of the preparer Φ(θP) a wavepacket narrow in angular distribution.
Another way to look at the problem is to note that we want to place the state of the particle at a precise position on the circle—if there is uncertainty in its positioning, as if it would be the case if θP were to have a large uncertainty, it will wash out the finer details of its space dependence, so we will not be able to see the short wavelength oscillations we are interested in. To ensure this, we need, again, to take for Φ(θP) a wavepacket narrow in angular distribution.
For an explicit example, let Φ(θP) be a top-hat function with spread 2η, i.e.,
Φ(θP)=12ηg(θP;η).
[21]
Then, the scalar product
PΦm|ΦmP=ππeimθPΦ(θP)eimθPΦ(θP)dθP=12ηηηeimθPeimθPdθP=sin((mm)η)(mm)η,
[22]
where we have used the angular representation eimθPΦ(θP) of |ΦmP.
Since in our case the angular momenta of interest are limited to the interval Nm,mN, the difference is bounded, |mm|2N. Hence, by choosing η small enough, we can make all the scalar products [22] as close to 1 as we wish and hence, from [20], the state of the particle as close to Ψ as we wish.

The Final State of the Preparer

We have now arrived at the crucial point of our paper. Although in our preparation stage we have not prepared the pure state Ψ, the state that we prepared has all the ingredients essential for our purpose:
The particle’s state has only angular momentum components in the interval [N,N]. Note that although the particle’s state is only an approximation of the pure state Ψ, the condition that there are no angular momentum components larger than N in its decompositions is strictly valid, as in Ψ.
By choosing η appropriately small, we can make the particle’s state approximate as well as we want the pure state Ψ. In particular, this new state of the particle presents the same superocillations as Ψ: In the region |θ|=O(1/N1/2+ϵ), it looks approximately like eiaNθ, corresponding to angular momentum aN, with a>1, larger than all angular momentum components in its decomposition.
Due to the above, in the subsequent stage of the experiment—the measurement stage—all will be as close as we want to what happens when starting with Ψ. That is, when the particle is found in the superoscillatory region, its angular momentum is close to aN, much larger than its maximal initial value of N. However, the measuring device does not provide the angular momentum difference to compensate for the increase of the particle’s angular momentum from its maximal initial value of N to around aN. More precisely, when the particle is found with angular momentum aN, the state of the measuring device does not change at all, so it does not give the particle any angular momentum whatsoever. When the particle is found with angular momentum different from aN (which occurs with nonnegligible probability only for deviations of order N1/2), the measuring device provides angular momentum to compensate for this difference, but not for the increase from the maximal initial value of N to aN. Hence, our paradoxical effect stands: The particle can emerge with an angular momentum much larger than any angular momentum in its initial state without the measuring device—the only system with which it interacted—to give it the difference.
Let’s now see what happens to the preparer.
At first sight, as far as angular momentum is concerned, the preparer’s role is rather trivial: It provides the angular momentum gained by the particle from its initial zero angular momentum state, |0p to the desired superposition. Indeed, that was the whole point of the previous section. As Eq. 20 shows, if after the preparation, we measure the angular momentum of the particle and find it to be m, meaning that the particle gained angular momentum m, then, the preparer is in the state |ΦmP, whose angular momentum probability distribution is identical to that in the initial state |ΦP, but shifted by m. This is a trivial case of angular momentum conservation, as discussed above.
Importantly for us here, since the particle’s state only has components limited to the interval [N,N], the preparer never provides more than angular momentum N (i.e., the maximal down-shift of the angular momentum distribution of the preparer is N).
Our experiment, however, requires that after preparation, we first check whether the particle is in the superoscillatory region, and only then we measure its angular momentum. So suppose we find the particle in a large spatial interval in the superoscillatory region and that the subsequent measurement of the particle’s angular momentum yields the value k. The preparer’s state in this situation is (up to normalization)
pk|Π̂|χp,P,
[23]
where Π̂ is the particle projection operator onto that interval.
To evaluate the preparer’s state, it is convenient to express |χp,P as
|χp,P=m=NNcm|mp|ΦmP=m=NNcmeimθ̂P|mp|ΦP=eiL̂θ̂Pm=NNcm|mp|ΦP=eiL̂θ̂P|Ψp|ΦP,
[24]
where L̂ is the particle angular momentum operator and θ̂P the particle angle operator.
Using [24] and the crucial fact that |ΦP, the initial state of the preparer, has only a very narrow angular distribution around θP=0, we obtain
pk|Π̂|χp,P=pk|Π̂eiL̂θ̂P|Ψp|ΦPpk|Π̂(1+iL̂θ̂P)|Ψp|ΦP=pk|Π̂|Ψp(1+ipk|Π̂L̂|Ψppk|Π̂|Ψpθ̂P)|ΦPpk|Π̂|Ψpeipk|Π̂L̂|Ψppk|Π̂|Ψpθ̂P|ΦP=pk|Π̂|Ψp|Φpk|Π̂L̂|Ψppk|Π̂|ΨpP,
[25]
where we used first-order approximations in the small angle θP.
The last line of Eq. 25 shows that (up to normalization), the final state of the preparer is equal to its initial state but displaced down in angular momentum by pk|Π̂L̂|Ψp/pk|Π̂|Ψp. Let us evaluate this quantity.
pk|Π̂L̂|Ψppk|Π̂|Ψp=supereikθ(i)Ψ(θ)θdθsupereikθΨ(θ)=supereikθ(i)θ(eiaNθ+O(1/N))dθsupereikθ(eiaNθ+O(1/N))dθ=aN+O(1/N).
[26]
Hence, the (normalized) state of the preparer, given that the particle was found in the superoscillatory region and that a subsequent measurement of its angular momentum found it to be equal to k is, up to O(1/N), equal to
|ΦaNP.
[27]
This is the key result of our paper. We will discuss its significance in the next sections, but before that, let us note a few more details. First, the final state of the preparer is not affected by the precise localization of the projected space interval in the superoscillation area. (That’s why we denoted the integration domain simply as “super” and not by indicating an exact location). This is important for our further analysis where we consider the projection being made by the interaction with the position-measuring device. As discussed before, the projection realized by the position measurement is not on some precise location on the circle, but on an interval centered around θM, the location of the measuring device. Even though we can make θM as precisely localized on the circle as we want, we can never achieve infinite precision, so the projection intervals will differ slightly from one another. Since it is not sensitive to the precise location of this space interval, our result about the final state of the preparer applies to all these particular projections.
Second, we note that the final state of the preparer is independent of the particular angular momentum value k with which we find the particle after localizing it in the superoscillatory region. In all the cases when the particle is found in the superoscillatory region, the final state of the preparer is the same, i.e. state given in Eq. [27].

A Second Nonconservation: “Preparation Nonconservation”

Let us now analyze our key result. What Eq. 27 shows is that in all of the cases where the particle was later found to be in the superoscillatory region, the final state of the preparer is equal to its initial state but shifted down in angular momentum by aN. That is, in all these cases, the preparer loses aN angular momentum. Yet, the particle started in the state of zero angular momentum, |0p and the preparation brings it in a state [20] whose angular momentum components are limited to the interval [N,N]. Thus, the angular momentum lost by the preparer is not transferred to the particle. We have found therefore another instance of angular momentum nonconservation in our cases of interest.
This “preparation nonconservation” is, if anything, more subtle than the nonconservation that occurs during the subsequent position measurement. The crucial point is that we cannot see this nonconservation right away but we have to wait until after the position measurement. Indeed, while there are, of course, many things we can find out immediately after the preparation, without any need to wait, they are not enough for spotting the preparation nonconservation. For example, we can, if we wish, certify that the particle has only angular momentum components in the interval [N,N]. In other words, we certify that at this stage, the particle did not receive any large momentum such as aN. Importantly, we can certify this without affecting the experiment. This can be done by simply measuring the projector on this low angular momentum subspace. Since the state of the particle is an eigenstate of this projector, this measurement will not affect our experiment at all. Furthermore, we also can, without waiting, measure the angular momentum that the preparer has after the preparation. Since the preparer finished its interaction with the particle, and never interacts with it again, this measurement does not affect our experiment either. What we cannot do right away after the preparation and have to wait until after the position measurement is to know whether the particle will be found in the superoscillatory region or not. Not knowing this, we do not know which of the individual runs of the experiment correspond to our case of interest; hence, we do not know which results of the measurement of the angular momentum of the preparer should be included.

Putting all Together: Overall Conservation

Let us now put everything together. Our entire experiment consists of the following:
PreparationMeasurementofpositionSelectionofcasesofparticleinthesuperoscillatoryregionMeasurementofangularmomentumofparticle.
[28]
To these we may add, between the preparation and position measurement, a verification that the particle angular momentum is restricted to the interval [N,N], i.e., measuring the projector on this interval.
The corresponding time evolution, restricting ourselves only to the cases when the particle is found at the end of the experiment in the superoscillatory region, is
|0p|ΦP|ϕM|χp,P|ϕM=m=NNcm|mp|ΦmP|ϕMk=sinc(kφ)|aN+kp|ΦaNP|ϕkM,
[29]
where the simple arrow “” describes unitary evolution while the double arrow “” describes unitary evolution plus selection, and φ is the size of the angular interval within the superoscillatory region onto which the position projection measurement is performed.
What the above equation shows is that the particle starts with zero angular momentum (i.e., in state |0p) and ends up gaining angular momentum aN+k, while the preparer provides aN and the position measuring device provides k. Yet, the preparation stage alone does not provide the particle with the high angular momentum aN: at the end of the preparation stage, the particle’s maximal angular momentum is only N.
This is the main result of our study:
The two nonconservation effects—the “preparation nonconservation” and the “measurement nonconservation”—compensate each other and lead to overall angular momentum conservation even when we restrict us to the subensemble of cases when the particle is found in the superoscillatory region. That is, conservation holds for these individual cases, not only statistically.

Discussion I

Let us now discuss the above result. First, there are three simple observations. Given that the particle is found in the superoscillatory region:
(i)
It is the preparer that delivers the angular momentum aN, allowing the particle to behave at the end of the experiment as a particle with genuine angular momentum aN.
(ii)
When after the position measurement the particle is found with angular momentum aN, the measuring device does not provide any angular momentum at all.
(iii)
When the particle is found with angular momentum different from aN, say aN+k, the position measuring device delivers angular momentum k. This is precisely what it would have done, had the particle been a genuine high angular momentum state before the position measurement, to account for the disturbance done to that monochromatic wave by truncating it to a finite wave train.
More importantly, this is not a simple conservation—it is the composite of two nonconservations. It also has a “holistic” time character: As we noticed before, by doing or not doing the position projection measurement, we can change the overall angular momentum transfer from the preparer to the particle, despite that a) at this stage, the particle and the preparer no longer interact and b) that we can certify that after the interaction with the preparer, the particle does not have any high angular momentum at all. This leads us to ask the following: Despite the overall conservation, where from and how precisely did the particle get the high angular momentum, if it did not have it before interacting with the position measuring device and the position measuring device did not change its state? Where has the high angular momentum lost by the preparer been stored until it finally materialized in the particle?
Note that both the preparer and the position measuring device play crucial roles: The preparer is the source of the high angular momentum gained by the particle, while the position measuring device gives an “umbrella” under which this transfer can occur at a time later than the one when the particle and the preparer interacted.
It is also instructive to contrast the above story with what happens in a related, but fundamentally different, case. Suppose that instead of preparing the particle in our special superposition, i.e., instead of the transformation [20], we simply use the preparer to prepare a state of well-defined angular momentum m, with NmN, and then subject it to the same experiment as before. That is, after preparation, we measure the projection operator on what previously was the superoscillatory region and, after that, if we found the particle in this region, we measure the angular momentum of the particle. In this region, the particle’s state oscillates with spatial frequency corresponding to the angular momentum m. Yet, after the truncation of the wavefunction, it is still possible to find the particle with angular momentum aN, much larger than its initial angular momentum m. This happens with a small probability, corresponding to the tail of the frequency probability due to truncation, but still, with nonzero probability. (Contrast this with the probability of finding the particle with momentum close to aN in the superoscillatory case given that we found the particle in this region which is close to 1.) Where did the particle get its angular momentum from now?
|0p|ΦP|ϕM|mp|ΦmP|ϕMk=ek|aN+kp|ΦmP|ϕ(aN+km)M,
[30]
with ek=sinc((aN+km)φ).
What we see here is a trivial case of angular momentum conservation. The particle gains angular momentum aN+k, by a two-stage process. In the first stage, it gains m, and the preparer provides it, by shifting its state to |ΦmP, i.e., down in angular momentum by m. There is no nonconservation now at this stage. In the second stage, the position measuring device disturbs this intermediate particle state and brings its angular momentum from m to aN+k, while losing itself aN+km, hence a trivial conservation again.
Coming back to our example, one can ask how is it possible that the position measurement and associated selection can affect what has happened to the preparer at an earlier time? Moreover, why does the preparer matter at all? After all, once a state, say |Ψ, is prepared, it does not matter how it was prepared. The answer is that in our modified experiment, we did not prepare a pure state. We have not prepared the special state |Ψ. What we have prepared is an entangled state |χp,P, [20], between the particle and the preparer, with the property that the reduced density matrix of the particle can be made as close as we want to the pure state Ψ. Nevertheless, the particle is entangled with the preparer. True, |χp,P is a very weakly entangled state: Each angular momentum component |mp is correlated with a corresponding preparer state |ΦmP which is identical to the initial state of the measuring device shifted in angular momentum by m. As discussed in the preparation section, we can make these states of the preparer as close to each other as we want, PΦm|ΦmP1, by making them wider and wider spread in angular momentum, so that |χp,P|Ψp|ΦP. This means that the state of the particle can be made as close as we want to the pure state Ψ. Hence, for its subsequent behavior, the particle behaves as close as we want to how it would in the pure state Ψ. Yet, for questions related to angular momentum conservation, there is an enormous difference between the entangled state |χp,P, and the pure state |Ψp|ΦP. Indeed, although the states |ΦmP can be made as close to each other as we want, their average angular momenta remain finitely different from each other, L0m versus L0m with L0 being the average angular momentum of |ΦP. This is the reason why this entanglement, while minimal, is however essential. It is essential even for the simple case when we just prepare the initial state |χp,P and then we immediately verify that the preparation conserves angular momentum. It is even more important in our special case. Postselecting for the particle being in the superoscillatory region and then for a particular final angular momentum produces a superposition of these shifted wavefunctions, which, by interference, lead to a wavefunction with a much larger shift in angular momentum, as discussed in the previous sections.
Of course, while the entanglement with the preparer explains the mathematical machinery that allows our results to exist, it is by no means, by itself, an explanation for why this effect happens. It does not tell why it is the case that this entanglement is exactly such that angular momentum conservation is valid for the individual cases when the particle is found in the superoscillatory region, while the only thing demanded by the standard conservation laws is statistical conservation over the entire ensemble. The main principle, as we see it, is that we should demand more of the conservation laws than the statistical conservation.

Discussions II. The Pure State Ψ(θ) Does Not Exist in Nature

One could, of course, try and bring a counterargument to our general line of thinking. One could ask what would happen if the particle were initially exactly in the pure state Ψ(θ)? Then, there would be no preparer to provide the required supplementary angular momentum, and we would not have angular momentum conservation in our individual case. Would this not invalidate our arguments?
Yes, if the particle could start in the initial state Ψ(θ), there would be genuine nonconservation in the individual cases presented in our original experiment, as described in ref. 1. It would then follow that conservation does not need to hold in individual cases but only statistically, no matter how unpalatable this may seem to us. But there is a way out. This brings us to the last key element of our paper. We claim that
The pure state Ψ(θ) is unphysical and does not exist in nature.
Arguing that Ψ(θ) is unphysical and does not exist in nature seems to contradict one of the basic postulates of quantum mechanics, namely that any normalized wavefunction is a legitimate state for a quantum particle. The answer is that the issue is one concerning frames of reference. The wavefunction Ψ(θ) has no meaning because the angle θ has, strictly speaking, no meaning.
It is standard in quantum mechanics to consider wavefunctions of variables x, y, z or of angle θ and so on. But it is well understood that what they do represent are not some absolute values, but they are coordinates measured relative to some frame of reference, say the walls of the laboratory. The reason why one does not always mention this explicitly is that in general this does not significantly affect the results and can be ignored. In our case, however, it matters significantly, as we have shown. The preparer acts as a reference frame, and this is why it should always be present.
Lest it appears that the statement that “we need to always use a frame of reference in quantum mechanics in order to correctly describe conservation laws” is trivial, we want to emphasize that this is by no means so. Far from it. It is in fact a very subtle issue, which only now is becoming apparent. Indeed, there is absolutely nothing in standard quantum mechanics that requires us to refer to a frame of reference to ensure that the usual, statistical conservation laws hold. Indeed, in the standard quantum mechanical formalism, nothing prevents us to write an arbitrary wavefunction of two particles, say Ψ(x1)Φ(x2), and as long as they interact via a potential that depends only on their relative distance, V(x1x2), the standard statistical momentum conservation law holds exactly. Nothing else is needed. There is no need to refer to any other frame of reference or any “preparation” device, etc. Similarly, no consideration of a reference frame is needed to ensure the statistical conservation of angular momentum or energy, etc., and they apply to all wavefunctions. We could, if we fancy doing so, refer all the position or time coordinates to some other physical system, but there is no need whatsoever to do it. What we found here is therefore a fundamental aspect of conservation laws:
If we insist on conservation at an individual level, we need to take the issue of frames of reference and of preparation devices into account, while this is not necessary if we only demand conservation at the statistical level.
Moreover, and crucially important, the mere thing that one needs a frame of reference, and hence a preparer, is only a necessary but by no means sufficient condition to imply conservation at the level of individual cases. This is by no means the “explanation” for the effect. What is required is the entire subtle interplay between the preparer and the particle and their nonlocal-in-time angular momentum transfer via the measuring device which acts as an umbrella that makes this transfer possible by covering otherwise inevitable causality violations.

Conclusions: The Meaning of Quantum Conservation Laws and the Basic Postulates of Quantum Mechanics

Let us zoom out from the particular example discussed here. We have argued that while the standard formulation of conservation laws in quantum mechanics, which is of a statistical nature, is perfectly valid as far as it goes, it is incomplete and needs to be revisited, specifically that we need to go beyond the statistical formulation and consider individual cases as well. In particular, we have argued that if we find in one particular run of an experiment, that, say, when we open a window of a box containing a single particle of energy strictly smaller than 1 eV and the particle emerges with energy of order of millions of GeV, it is legitimate to ask where did this increase in energy come from in this individual case. Had we ignored this question on grounds that the standard, statistical, conservation law is all there is, we would have not identified the strange conservation effect for the individual case presented here, and hence missed a lot of interesting physics. We would have also missed the implications for the need to explicitly take into account the issue of the frames of reference involved in the preparation of the initial state, an issue which does not arise when only the standard statistical conservation law is concerned but which arises when the conservation in individual cases is concerned, neither the fact that certain quantum states are unphysical, while there would be considered perfectly valid in standard quantum mechanics. We take this as a good indicator of the validity of this line of enquiry and believe these results are only the tip of an iceberg, part of a more general structure concerning conservation laws. In particular, we conjecture that when such a full analysis of any conservation experiment is performed conservation is obeyed in any individual case, not only statistically.

Data, Materials, and Software Availability

There are no data underlying this work.

Acknowledgments

S.P. acknowledges the support of the Advanced European Research Council (ERC) Grant FLQuant.

Author contributions

Y.A., S.P., and D.R. performed research; and S.P. wrote the paper.

Competing interests

The authors declare no competing interest.

Supporting Information

Appendix 01 (PDF)

References

1
Y. Aharonov, S. Popescu, D. Rohrlich, On conservation laws in quantum mechanics. Proc. Natl. Acad. Sci. U.S.A. 118, e1921529118 (2021).
2
Y. Aharonov, S. Popescu, D. Rohrlich, Tel Aviv University Preprint TAUP 847-90 (1991). S. Popescu, PhD Thesis, Tel Aviv University (1991).
3
M. V. Berry, “Faster than Fourier” in Quantum Coherence and Reality in Celebration of the 60th Birthday of Yakir Aharonov, J. S. Anandan, J. L. Safko, Eds. (World-Scientific, Singapore, 1994), pp. 55–65.
4
M. V. Berry, S. Popescu, Evolution of quantum superoscillations and optical superresolution without evanescent waves. J. Phys. Math. Gen. 39, 6965 (2006).
5
Y. Aharonov, F. Colombo, I. Sabadini, D. C. Struppa, J. Tollaksen, Superoscillating sequences as solutions of generalized Schrödinger equations. J. Math. Pure Appl. 103, 522 (2015).
6
M. V. Berry et al., Roadmap on superoscillations. J. Optics 21, 053002 (2019).

Information & Authors

Information

Published in

The cover image for PNAS Vol.120; No.41
Proceedings of the National Academy of Sciences
Vol. 120 | No. 41
October 10, 2023
PubMed: 37782805

Classifications

Data, Materials, and Software Availability

There are no data underlying this work.

Submission history

Received: December 9, 2022
Accepted: July 31, 2023
Published online: October 2, 2023
Published in issue: October 10, 2023

Keywords

  1. quantum mechanics
  2. foundations
  3. conservation laws

Acknowledgments

S.P. acknowledges the support of the Advanced European Research Council (ERC) Grant FLQuant.
Author contributions
Y.A., S.P., and D.R. performed research; and S.P. wrote the paper.
Competing interests
The authors declare no competing interest.

Notes

Reviewers: L.H., Perimeter Institute; and S.M., Université Libre de Bruxelles.

Authors

Affiliations

Yakir Aharonov1 [email protected]
School of Physics and Astronomy, Tel Aviv University, Tel Aviv 69978, Israel
Institute for Quantum Studies, Chapman University, Orange, CA 92866
Department of Physics, Schmid College of Science and Technology, Chapman University, Orange, CA 92866
Sandu Popescu1 [email protected]
H. H. Wills Physics Laboratory, University of Bristol, Bristol BS8 1TL, United Kingdom
Physics Department, Ben-Gurion University of the Negev, Beersheba 8410501, Israel

Notes

1
To whom correspondence may be addressed. Email: [email protected] or [email protected].

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    Conservation laws and the foundations of quantum mechanics
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