Abstract

The reduced chain entanglement of brush polymers over their linear analogs drastically lowers the energetic barriers to reorganization. In this report, we demonstrate the rapid self-assembly of brush block copolymers to nanostructures with photonic bandgaps spanning the entire visible spectrum, from ultraviolet (UV) to near infrared (NIR). Linear relationships were observed between the peak wavelengths of reflection and polymer molecular weights. This work enables “bottom-up” fabrication of photonic crystals with application-tailored bandgaps, through synthetic control of the polymer molecular weight and the method of self-assembly. These polymers could be developed into NIR-reflective paints, to combat the “urban heat island effect” due to NIR photon thermalization.

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ACKNOWLEDGMENTS.

This work was supported by the NSF (CHE-1048404). R.A.W. was supported in part by the DOE “Light-Material Interactions in Energy Conversion” Energy Frontier Research Center (DE-SC0001293). R.A.W. thanks the Resnick Institute for a graduate fellowship. Reflection measurements were collected at the Molecular Materials Research Center of the Beckman Institute of the California Institute of Technology. We thank Zhen-Gang Wang for helpful discussions and Bryce Sadtler for assistance with the reflection measurements.

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Information & Authors

Information

Published in

The cover image for PNAS Vol.109; No.36
Proceedings of the National Academy of Sciences
Vol. 109 | No. 36
September 4, 2012
PubMed: 22912408

Classifications

Submission history

Published online: August 21, 2012
Published in issue: September 4, 2012

Acknowledgments

This work was supported by the NSF (CHE-1048404). R.A.W. was supported in part by the DOE “Light-Material Interactions in Energy Conversion” Energy Frontier Research Center (DE-SC0001293). R.A.W. thanks the Resnick Institute for a graduate fellowship. Reflection measurements were collected at the Molecular Materials Research Center of the Beckman Institute of the California Institute of Technology. We thank Zhen-Gang Wang for helpful discussions and Bryce Sadtler for assistance with the reflection measurements.

Authors

Affiliations

Benjamin R. Sveinbjörnsson1
Arnold and Mabel Beckman Laboratories for Chemical Synthesis, Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125; and
Raymond A. Weitekamp1
Arnold and Mabel Beckman Laboratories for Chemical Synthesis, Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125; and
Thomas J. Watson Laboratories of Applied Physics, California Institute of Technology, Pasadena, CA 91125
Garret M. Miyake
Arnold and Mabel Beckman Laboratories for Chemical Synthesis, Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125; and
Yan Xia
Arnold and Mabel Beckman Laboratories for Chemical Synthesis, Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125; and
Harry A. Atwater
Thomas J. Watson Laboratories of Applied Physics, California Institute of Technology, Pasadena, CA 91125
Robert H. Grubbs2 [email protected]
Arnold and Mabel Beckman Laboratories for Chemical Synthesis, Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125; and

Notes

2
To whom correspondence should be addressed, E-mail: [email protected].
Contributed by Robert H. Grubbs, July 30, 2012 (sent for review July 3, 2012)
Author contributions: R.A.W., Y.X., and R.H.G. designed research; B.R.S., R.A.W., G.M.M., and Y.X. performed research; B.R.S. contributed new reagents/analytic tools; B.R.S., R.A.W., G.M.M., Y.X., and H.A.A. analyzed data; and B.R.S., R.A.W., G.M.M., Y.X., H.A.A., and R.H.G. wrote the paper.
1
B.R.S. and R.A.W. contributed equally to this work.

Competing Interests

The authors declare no conflict of interest.

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    Rapid self-assembly of brush block copolymers to photonic crystals
    Proceedings of the National Academy of Sciences
    • Vol. 109
    • No. 36
    • pp. 14281-14716

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