Structural genes of wheat and barley 5-methylcytosine DNA glycosylases and their potential applications for human health

Contributed by Diter von Wettstein, October 15, 2012 (sent for review October 5, 2012)
November 26, 2012
109 (50) 20543-20548

Abstract

Wheat supplies about 20% of the total food calories consumed worldwide and is a national staple in many countries. Besides being a key source of plant proteins, it is also a major cause of many diet-induced health issues, especially celiac disease. The only effective treatment for this disease is a total gluten-free diet. The present report describes an effort to develop a natural dietary therapy for this disorder by transcriptional suppression of wheat DEMETER (DME) homeologs using RNA interference. DME encodes a 5-methylcytosine DNA glycosylase responsible for transcriptional derepression of gliadins and low-molecular-weight glutenins (LMWgs) by active demethylation of their promoters in the wheat endosperm. Previous research has demonstrated these proteins to be the major source of immunogenic epitopes. In this research, barley and wheat DME genes were cloned and localized on the syntenous chromosomes. Nucleotide diversity among DME homeologs was studied and used for their virtual transcript profiling. Functional conservation of DME enzyme was confirmed by comparing the motif and domain structure within and across the plant kingdom. Presence and absence of CpG islands in prolamin gene sequences was studied as a hallmark of hypo- and hypermethylation, respectively. Finally the epigenetic influence of DME silencing on accumulation of LMWgs and gliadins was studied using 20 transformants expressing hairpin RNA in their endosperm. These transformants showed up to 85.6% suppression in DME transcript abundance and up to 76.4% reduction in the amount of immunogenic prolamins, demonstrating the possibility of developing wheat varieties compatible for the celiac patients.

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Data Availability

Data deposition: The sequences reported in this paper have been deposited in the GenBank database (accession nos. FM164415.1, JF683316, JF683317, and JF683318).

Acknowledgments

We thank P. Reisenauer and E. Mackenzie and Drs. N. Ankrah, J. L. Ullman, and R. Brueggeman for field and laboratory assistance. This work was supported by National Institutes of Health Grants GM080749-01A2 and 2R42DK072721-02, Life Sciences Discovery Fund Grant 3143956, a Mercator Professorship from the German Research Foundation (to D.v.W.), and Programme of Introducing Talents of Discipline to Universities Project B07017 to Key Laboratory of Vegetation Ecology, Ministry of Education, People's Republic of China.

Supporting Information

Supporting Information (PDF)
Supporting Information
sd01.xlsx
sd02.xlsx

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Information & Authors

Information

Published in

The cover image for PNAS Vol.109; No.50
Proceedings of the National Academy of Sciences
Vol. 109 | No. 50
December 11, 2012
PubMed: 23184965

Classifications

Data Availability

Data deposition: The sequences reported in this paper have been deposited in the GenBank database (accession nos. FM164415.1, JF683316, JF683317, and JF683318).

Submission history

Published online: November 26, 2012
Published in issue: December 11, 2012

Keywords

  1. gluten intolerance
  2. autoimmune reaction
  3. prophylactic measure

Acknowledgments

We thank P. Reisenauer and E. Mackenzie and Drs. N. Ankrah, J. L. Ullman, and R. Brueggeman for field and laboratory assistance. This work was supported by National Institutes of Health Grants GM080749-01A2 and 2R42DK072721-02, Life Sciences Discovery Fund Grant 3143956, a Mercator Professorship from the German Research Foundation (to D.v.W.), and Programme of Introducing Talents of Discipline to Universities Project B07017 to Key Laboratory of Vegetation Ecology, Ministry of Education, People's Republic of China.

Authors

Affiliations

Shanshan Wen
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Key Laboratory of Molecular Epigenetics of the Ministry of Education, Northeast Normal University, Changchun 130024, China;
Nuan Wen
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Jinsong Pang
Key Laboratory of Molecular Epigenetics of the Ministry of Education, Northeast Normal University, Changchun 130024, China;
Gregor Langen
Division Phytopathology, Institute of Phytopathology and Applied Zoology, Justus Liebig University, D-35392 Giessen, Germany;
Rhoda A. T. Brew-Appiah
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Jaime H. Mejias
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Claudia Osorio
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Mingming Yang
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Richa Gemini
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
Charles P. Moehs
Arcadia Biosciences, Seattle, WA 98119;
Robert S. Zemetra
Department of Crop and Soil Science, Oregon State University, Corvallis, OR 97331; and
Karl-Heinz Kogel
Division Phytopathology, Institute of Phytopathology and Applied Zoology, Justus Liebig University, D-35392 Giessen, Germany;
Bao Liu
Key Laboratory of Molecular Epigenetics of the Ministry of Education, Northeast Normal University, Changchun 130024, China;
Xingzhi Wang1 [email protected]
Key Laboratory of Molecular Epigenetics of the Ministry of Education, Northeast Normal University, Changchun 130024, China;
Diter von Wettstein1 [email protected]
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;
School of Molecular Biosciences, Washington State University, Pullman, WA 99164
Sachin Rustgi1 [email protected]
Department of Crop and Soil Sciences, Washington State University, Pullman, WA 99164;

Notes

1
To whom correspondence may be addressed. E-mail: [email protected], [email protected], or [email protected].
Author contributions: D.v.W. and S.R. designed research; S.W., N.W., J.P., G.L., R.A.T.B.-A., J.H.M., C.O., M.Y., and S.R. performed research; C.P.M., R.S.Z., K.-H.K., B.L., and X.W. contributed new reagents/analytic tools; S.W., R.G., and S.R. analyzed data; and S.W., D.v.W., and S.R. wrote the paper.

Competing Interests

The authors declare no conflict of interest.

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    Structural genes of wheat and barley 5-methylcytosine DNA glycosylases and their potential applications for human health
    Proceedings of the National Academy of Sciences
    • Vol. 109
    • No. 50
    • pp. 20167-20774

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